1961—Shortly after the invention of the ruby laser, Don Jennings built and operated the first ruby laser at NIST. The lasing effect was achieved with a small ruby crystal, 1/4 inch in diameter and 1 and 1/4 inches long. The ends were optically polished flat and parallel and coated with silver. The crystal was optically excited from the sides by a xenon flash lamp built by George Unger in the NIST chemistry glass shop.
1963—NIST scientists Don Jennings and Jan Hall designed a ruby laser that could be focused down to an intense, uniform, pinpoint beam just 20 micrometers in diameter. They used this laser to conduct one of the first nonlinear absorption experiments, using anthracene crystals. Nonlinear absorption is a process in which two particles of light (photons) are absorbed simultaneously, exciting an atom by an amount of energy equal to the sum of the two photon energies. When the crystals were excited by ruby laser light, they emitted intense blue fluorescence (a shorter wavelength of light). The revolutionary result broke Stokes Law, which held that the fluorescence wavelength was always longer than the excitation wavelength.
1965—The first quantitative and predictable "two-photon detachment" was performed by NIST scientist Jan Hall working with Lewis Branscomb using a ruby laser and a beam of negative iodine molecules. The experiment provided a clear validation of the new technique of detaching electrons from atoms using two photons of laser light. The technique has led to advances in a wide range of technology areas, from radar performance to quantum cryptography, the most secure method known for protecting the privacy of a communications channel.
Mid-1960s—NIST researchers made many groundbreaking laser-based distance measurements, which eventually led to a number of world-record measurements of the speed of light and redefinition of the meter in terms of the speed of light. The work began in the Poorman's Relief Gold Mine in Colorado, which offered a steady temperature and a 40-meter-long straight path enabling accurate laser frequency measurements. A stable 30-meter-long vacuum interferometer was built to study the interference patterns created by light waves. This led to the invention of a way to stabilize lasers by locking them to a frequency that induced a transition between specific energy levels in molecules such as methane and iodine. In addition, the laser-based distance measurements made in the gold mine were converted by NIST researcher Judah Levine into measurements of the Earth's movement, which turned out to be one way of supporting the detection and measurement of underground nuclear tests by the United States and Russia. Levine also obtained new data about the state of the Earth's liquid core by monitoring the stretching of the Earth produced by the tidal effects of the sun and moon.
1966—NIST began its program to develop measurement tools for lasers. Early demands for laser power and energy measurements were driven by military applications and civilian laser safety concerns. Some of the earliest work focusing on laser safety issues helped to accelerate the dissemination of everyday laser products, such as grocery store scanners. Each advance required new types of measurements to verify performance and enable manufacturers to produce a uniform product. NIST initially focused on developing standard calorimeters to measure the power in laser beams. For instance, NIST built calorimeters to measure the output of very high-energy lasers to be used in defensive weapons of the Strategic Defense Initiative ("Star Wars") program. The early capabilities developed at NIST supported industrial-safety measurements of the laser pointers used in lecture presentations.
1967—NIST provides its first calibration of laser power for an industrial customer.
1969—James Faller of NIST first suggested that astronauts place reflectors on the moon. Faller also provided the initial designs for the first reflector array and two subsequent arrays. By measuring the round-trip travel time for a laser pulse sent to the moon and reflected back (about 2.5 seconds), other scientists measured the distance between the Earth and moon to better than 2.5 cm (1 inch). Experiments with lunar laser ranging instruments are still active today and are credited with dramatically increasing understanding of Earth and moon geophysics and dynamics as well as gravitational physics.