Major Leap for Nuclear Clock Paves Way for Ultraprecise Timekeeping

The world keeps time with the ticks of atomic clocks, but a new type of clock under development — a nuclear clock — could revolutionize how we measure time and probe fundamental physics.

An international research team led by scientists at JILA, a joint institute of the National Institute of Standards and Technology (NIST) and the University of Colorado Boulder, has demonstrated key elements of a nuclear clock. A nuclear clock is a novel type of timekeeping device that would use signals from the core, or nucleus, of an atom. The team used a specially designed ultraviolet laser to precisely measure the frequency of an energy jump in thorium nuclei embedded in a solid crystal. They also employed an optical frequency comb, which acts like an extremely accurate light ruler, to count the number of ultraviolet wave cycles that create this energy jump. While this laboratory demonstration is not a fully developed nuclear clock, it contains all the key technology for one.

Nuclear clocks could be much more accurate than current atomic clocks, which provide official international time and play major roles in technologies and applications such as GPS and internet synchronization, and in financial transactions. For the general public, this development could ultimately mean even more precise navigation systems (with or without GPS), faster internet speeds, more reliable network connections, and more secure digital communications. 

Beyond everyday technology, nuclear clocks could improve tests of fundamental theories for how the universe works, potentially leading to new discoveries in physics. They could help detect dark matter or verify if the constants of nature are truly constant, allowing for verification of theories in particle physics without the need for large-scale particle accelerator facilities.

Laser Precision in Timekeeping

Atomic clocks measure time by tuning laser light to frequencies that cause electrons to jump between energy levels. Nuclear clocks would use energy jumps within an atom’s tiny central region, known as the nucleus, where particles called protons and neutrons cram together. These energy jumps are much like flipping a light switch. Shining laser light with the exact amount of energy needed for this jump can flip this nuclear "switch."

A nuclear clock would have major advantages for clock precision. Compared with the electrons in atomic clocks, the nucleus is much less affected by outside disturbances such as stray electromagnetic fields. The laser light needed to cause energy jumps in nuclei is much higher in frequency than that required for atomic clocks. This higher frequency — meaning more wave cycles per second — is directly related to a greater number of “ticks” per second and therefore leads to more precise timekeeping.

But it is very hard to create a nuclear clock. To make energy jumps, most atomic nuclei need to be hit by coherent X-rays (a high-frequency form of light) with energies much greater than those that can be produced with current technology. So scientists have focused on thorium-229, an atom whose nucleus has a smaller energy jump than any other known atom, requiring ultraviolet light (which is lower in energy than X-rays).

In 1976, scientists discovered this thorium energy jump, known as a “nuclear transition” in physics language. In 2003, scientists proposed using this transition to create a clock, and but they didn’t directly observe it until 2016. Earlier this year, two different research teams used ultraviolet lasers they created in the lab to flip the nuclear “switch” and measure the wavelength of light needed for it.

In the new work, the JILA researchers and their colleagues create all the essential parts of a clock: the thorium-229 nuclear transition to provide the clock's “ticks,” a laser to create precise energy jumps between the individual quantum states of the nucleus, and a frequency comb for direct measurements of these “ticks.” This effort has achieved a level of precision that is one million times higher than the previous wavelength-based measurement. In addition, they compared this ultraviolet frequency directly to the optical frequency used in one of the world's most accurate atomic clocks, which uses strontium atoms, establishing the first direct frequency link between a nuclear transition and an atomic clock. This direct frequency link and increase in precision are a crucial step in developing the nuclear clock and integrating it with existing timekeeping systems.

The research has already yielded unprecedented results, including the ability to observe details in the thorium nucleus's shape that no one had ever observed before — it’s like seeing individual blades of grass from an airplane.

The team presents its results in the Sept. 4 issue of the journal Nature as a cover story.

Toward a Nuclear Future

While this isn't yet a functioning nuclear clock, it is a crucial step toward creating such a clock that could be both portable and highly stable. The use of thorium embedded in a solid crystal, combined with the nucleus’s reduced sensitivity to external disturbances, paves the way for potentially compact and robust timekeeping devices.

“Imagine a wristwatch that wouldn't lose a second even if you left it running for billions of years,” said NIST and JILA physicist Jun Ye. “While we're not quite there yet, this research brings us closer to that level of precision.”

The research team included researchers from JILA, the Vienna Center for Quantum Science and Technology, and IMRA America Inc. 

Paper: Chuankun Zhang, Tian Ooi, Jacob S. Higgins, Jack F. Doyle, Lars von der Wense, Kjeld Beeks, Adrian Leitner, Georgy Kazakov, Peng Li, Peter G. Thirolf, Thorsten Schumm and Jun Ye. Frequency ratio of the ^229mTh nuclear isomeric transition and the ⁸⁷Sr atomic clock. Nature. Published online Sept 4, 2024. DOI: 10.1038/s41586-024-07839-6