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Search Publications by: Collin L. Broholm (Assoc)

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Displaying 1 - 25 of 66

Time evolution of a pumped molecular magnet - a time resolved inelastic neutron scattering study

January 1, 2025
Author(s)
T. Reeder, Paraj Titum, J. Kindervater, Qiang Ye, Jose Rodriguez Rivera, Yiming Qiu, Nicholas C. Maliszewskyj, T. McQueen, Collin L. Broholm
ntroducing an experimental technique of time-resolved inelastic neutron scattering (TRINS), we explore the time-dependent effects of resonant pulsed microwaves on the molecular magnet Cr8F8Piv16. The octagonal rings of magnetic Cr3+ atoms with

Intertwined Charge and Spin Density Waves in a Topological Kagome Material

July 22, 2024
Author(s)
Y. Chen, Jonathan N. Gaudet, G. Marcus, T. Nomoto, T. Chen, T. Tomita, M. Ikhlas, H. Suzuki, Yang Zhao, Wangchun Chen, J. Strempfer, R. Arita, S. Nakatsuji, Collin L. Broholm
Using neutrons and x rays we show the topological kagome antiferromagnet Mn3Sn for T 285 K forms a homogeneous spin and charge ordered state comprising a longitudinally polarized spin density wave with wave vector kβ = kβ ˆc, a helical modulated version

Continuum of magnetic excitations in the Kitaev honeycomb iridate D3LiIr2O6

February 12, 2024
Author(s)
Thomas Halloran, Yishu Wang, Kemp Plumb, M. B. Stone, Barry Winn, M. K. Graves-Brook, Jose Rodriguez Rivera, Yiming Qiu, Prashant Chauhan, N. Armitage, Tomohiro Takayama, Hidenori Takagi, Collin L. Broholm
Inelastic neutron scattering (INS) measurements of powder D3(7Li)(193Ir)2O6 reveal low energy magnetic excitations with a scattering cross section that is featureless versus |Q| and consistent with a Kitaev spin-liquid (KSL) state. The magnetic nature of

Noncollinear 2k Antiferromagnetism in the Zintl Semiconductor Eu5In2Sb6

January 29, 2024
Author(s)
Vincent Morano, Jonathan N. Gaudet, Nicodemos Varnava, Tanya Berry, Thomas Halloran, Chris Lygouras, Xiaoping Wang, Christina M. Hoffman, Guangyong Xu, Jeffrey Lynn, Tyrel McQueen, David Vanderbilt, Collin L. Broholm
Eu5In2Sb6 is an orthorhombic non-symmorphic small band gap semiconductor with three distinct Eu2+ sites and two low-temperature magnetic phase transitions. The material displays one of the greatest (negative) magnetoresistances of known stoichiometric

Spin-orbital order and excitons in magnetoresistive HoBi

March 22, 2023
Author(s)
Jonathan N. Gaudet, H. Yang, E. Smith, T. Halloran, J. Clancy, Jose Rodriguez Rivera, Guangyong Xu, Yang Zhao, Wangchun Chen, G. Sala, Adam A. Aczel, B. Gaulin, Fazel Tafti, Collin L. Broholm
The magnetism of the rock-salt fcc rare-earth monopnictide HoBi, a candidate topological material with extreme magnetoresistance, is investigated. From the Ho3+ non-Kramers J=8 spin-orbital multiplet, the cubic crystal electric field yields six near

Geometrical Frustration Versus Kitaev Interactions in BaCo 2 (AsO 4 ) 2

January 10, 2023
Author(s)
Thomas Halloran, Felix Desrochers, Emily Zhang, Tong Chen, Li E. Chern, Zhijun Xu, Barry Winn, Melissa Graves-Brook, M. B. Stone, Alexander I. Kolesnikov, Yiming Qiu, Ruidan Zhong, Robert Cava, Yong Kim, Collin L. Broholm
Recently, Co-based honeycomb magnets have been proposed as promising candidate materials to host the Kitaev spin liquid state. One of the front-runners is BaCo 2(AsO 4) 2 (BCAO), where it was suggested that the exchange processes between Co 2+ ions via the

Weyl-mediated helical magnetism in NdAlSi

August 19, 2021
Author(s)
Jonathan Gaudet, Hung-Yu Yang, Santu Baidya, Baozhu Lu, Guangyong Xu, Yang Zhao, Jose Rodriguez Rivera, Christina M. Hoffman, David E. Graf, Darius H. Torchinsky, Predrag Nikolic, David Vanderbilt, Fazel Tafti, Collin L. Broholm
Emergent relativistic quasiparticles in Weyl semimetals are the source of exotic electronic properties such as surface Fermi arcs, the anomalous Hall effect and negative magnetoresistance, all observed in real materials. Whereas these phenomena highlight

Monopolar and dipolar relaxation in spin ice Ho2Ti2O7

June 16, 2021
Author(s)
Yishu Wang, T. Reeder, Y. Karaki, J. Kindervater, T. Halloran, Nicholas C. Maliszewskyj, Yiming Qiu, Jose Rodriguez Rivera, Sergiy Gladchenko, S. M. Koohpayeh, S. Nakatsuji, Collin L. Broholm
Ferromagnetically interacting Ising spins on the pyrochlore lattice of corner-sharing tetrahedra form a highly degenerate manifold of low-energy states. A spin flip relative to this "spin-ice" manifold can fractionalize into two oppositely charged magnetic

Pristine Quantum Criticality in a Kondo Semimetal

May 19, 2021
Author(s)
Wesley T. Fuhrman, Andrey Sidorenko, Jonathan Hanel, Hannes Winkler, Andrey Prokofiev, Jose Rodriguez Rivera, Yiming Qiu, Peter Blaha, Qimiao Si, Collin L. Broholm, Silke Paschen
The observation of quantum criticality in diverse classes of strongly correlated electron systems has been instrumental in establishing ordering principles, discovering new phases, and identifying the relevant degrees of freedom and interactions. At focus

Noncollinear Ferromagnetic Weyl Semimetal with Anisotropic Anomalous Hall Effect

March 24, 2021
Author(s)
Hung-Yu Yang, Bahadur Singh, Jonathan Gaudet, Baozhu Lu, Cheng-Yi Huang, Wei-Chi Chiu, Shin-Ming Huang, Baokai Wang, Faranak Bahrami, Bochao Xu, Jacob Franklin, Ilya Sochnikov, David Graf, Guangyong Xu, Yang Zhao, Christina Hoffman, Hsin Lin, Darius Torchinsky, Collin L. Broholm, Arun Bansil, Fazel Tafti

Multiphase Magnetism in Yb 2 Ti 2 O 7

November 3, 2020
Author(s)
Allen Scheie, Jonas Kindervater, Shu Zhang, Hitesh Changlani, G. Sala, Georg Ehlers, Andre Heinemann, Gregory Tucker, Seyed Koohpayeh, Collin L. Broholm

Antichiral Spin Order, its Soft Modes, and their Hybridization with Phonons in the Topological Semimetal Mn 3 Ge

August 3, 2020
Author(s)
Y. Chen, Jonathan Gaudet, S. Dasgupta, G. G. Marcus, J. Lin, T. Chen, T. Tomita, M. Ikhlas, Yang Zhao, Wangchun Chen, Matthew B. Stone, O. Tchernyshyov, S. Nakatsuji, Collin L. Broholm
Quantum materials with strong transport responses to disparate physical quantities are of great fundamental significance and may hold technological potentials. The interplay between interactions and topology drive such responses through the effects of

Orientation Dependence of the Magnetic Phase Diagram of Yb 2 Ti 2 O 7

May 21, 2020
Author(s)
S. Saubert, A. Scheie, C. Duvinage, J. Kindervater, S. Zhang, H. J. Changlani, Guangyong Xu, S. M. Koohpayeh, O. Tchernyshyov, Collin L. Broholm, C. Pfleiderer
In the quest to realize a quantum spin liquid (QSL), magnetic long-range order is hardly welcome. Yet it can offer deep insights into a complex world of strong correlations and fluctuations. Much hope was placed in the cubic pyrochlore Yb 2Ti 2O 7 as a

Anisotropic Effect of a Magnetic Field on the Neutron Spin Resonance in FeSe

April 16, 2020
Author(s)
Tong Chen, Youzhe Chen, David W. Tam, Bin Gao, Yiming Qiu, Astrid Schneidewind, Igor Radelytskyi, Karel Prokes, Songxue Chi, Masaaki Matsuda, Collin L. Broholm, Pengcheng Dai
We use inelastic neutron scattering to study the effect of a magnetic field on the neutron spin resonance (Er = 3.6 meV) of superconducting FeSe (Tc = 9 K). While a field aligned along the in-plane direction broadens and suppresses the resonance, a c-axis

Low-Energy Magnons in the Chiral Ferrimagnet Cu 2 OSeO 3 : A Coarse-Grained Approach

April 8, 2020
Author(s)
Yi Luo, G. G. Marcus, Benjamin Trump, J. Kindervater, M. B. Stone, Jose Rodriguez Rivera, Yiming Qiu, T. M. McQueen, O. Tchernyshyov, Collin L. Broholm
We report a comprehensive neutron scattering study of low energy magnetic excitations in the breathing pyrochlore helimagnetic Cu 2OSeO 3. Fully documenting the four lowest energy magnetic modes that leave the ferrimagnetic configuration of the "strong

Homogeneous Reduced Moment in a Gapful Scalar Chiral Kagome Antiferromagnet

July 12, 2019
Author(s)
A. Scheie, S. Dasgupta, M. Sanders, A. Sakai, Y. Matsumoto, Timothy R Prisk, S. Nakatsuji, R. J. Cava, Collin L. Broholm
We present a quantitative experimental investigation of the scalar chiral magnetic order with in Nd 3Sb 3Mg 2O 14. Static magnetization reveals a net ferromagnetic ground state, and inelastic neutron scattering from the hyperfine coupled nuclear spin